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    Intermediate scattering potential strength in electron-irradiated YBa2Cu3O7−δ from London penetration depth measurements

    Kyuil Cho1,2, M. Kończykowski3, S. Teknowijoyo1,2, S. Ghimire1,2, M. A. Tanatar1,2, Vivek Mishra4, and R. Prozorov1,2,*

    • 1Ames Laboratory, Ames, IA 50011, USA
    • 2Department of Physics & Astronomy, Iowa State University, Ames, IA 50011, USA
    • 3Laboratoire des Solides Irradiés, École Polytechnique, CNRS, CEA, Institut Polytechnique de Paris, F-91128 Palaiseau, France
    • 4Kavli Institute for Theoretical Sciences, University of Chinese Academy of Sciences, Beijing 100190, China

    • *Corresponding author: prozorov@ameslab.gov

    Phys. Rev. B 105, 014514 – Published 25 January, 2022

    DOI: https://doi.org/10.1103/PhysRevB.105.014514

    Abstract

    Temperature-dependent London penetration depth, λ(T), of a high quality optimally doped YBa2Cu3O7−δ single crystal was measured using a tunnel-diode resonator. Controlled artificial disorder was induced at a low temperature of 20 K by 2.5 MeV electron irradiation with the accumulation of large doses of 3.8×1019 and 5.3×1019 electrons per cm2. The irradiation caused significant suppression of the superconductor's critical temperature, Tc, from 94.6 to 90.0 K and then to 78.7 K, respectively. The low-temperature behavior of λ(T) evolves from a Tlinear in pristine state to a T2behavior after the irradiation, expected for a line-nodal d-wave superconductor. However, the original theory that explained such behavior had assumed a unitary limit of the scattering potential, whereas usually in normal metals and semiconductors, Born scattering is sufficient to describe the experiment. To estimate the scattering potential strength, we calculated the normalized superfluid density, ρs(t=T/Tc)=λ2(0)/λ2(t), varying the amount and the strength of nonmagnetic scattering using a self-consistent t-matrix theory. Fitting the obtained curves to a power law, ρs=1−Rtn, and to a polynomial, ρs=1−At−Bt2, and comparing the coefficients n in one set and A and B in another with the experimental values, we estimate the phase shift to be around 70 and 65∘, respectively. We correlate this result with the evolution of the density of states with nonmagnetic disorder.

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